I really liked how flashy Dean & Rebecca's combo attack was in Wild Arms 5. I mean, the backflip over him was totally unnecessary. They go back to shooting exactly how they were before, but it just looks so cool.
Izuna Drop in Ninja Gaiden. I can't find a gif of it
Of late, I love the cat dive in 3DWorld. So satisfying to use, it's essentially a dive kick in a platformer
Stealth kills in Mark of the Ninja are also very fun and have a satisfying component.
And historically, I've enjoyed Sabin's Blitz moves in FFVI.
I was a big FG fan at the time, with SFII arcade being still pretty popular, so having SF commands was a fun mechanic in an RPG.
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Holy shit I'd never even heard of this game, I YT'ed a video of this clip and found a whole video with crazy attacks. I gotta try out this game.
http://www.youtube.com/watch?v=DqMAed1EAQU
From Wonderful 101 - spoiler heavy
Final Ultimate Legendary Earth Power Super Max Justice Future Miracle Dream Beautiful Galaxy Big Bang Little Bang Sunrise Starlight Infinite Fabulous Totally Final Wonderful Arrow... Fire!
Zandatsu.
Because it's a special move that can be different every time.
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Also, K's Chain Drive (KOF XIII) is fucking amazing. (Can't find gif).
http://www.youtube.com/watch?v=sub_1mAxNOw
Where the heck is SRT in this thread (only one in the first page, we need more)?
I give a nod to DaiRaiOh's Jinrai (Alpha 3 was the first time I ever did imports, so it holds a special place when it comes to SR series)
Runner up is NeoGranzon (all of its attacks) cause Shu is a badass
Honestly it's hard to narrow down my favorite attacks from the SR series (heck even the GBA versions have pretty good special attacks)
Why? The animation is orgasmic in the later entries of this series. You thought KoTR in FF7 was long then you haven't played enough SRW with animations on
Tiger Uppercut has one of the crunchiest animations ever, that makes it look powerful. Can't find a GIF ATM.
Not close to my favourite, but what first came to mind when I saw the thread title.
Uchiha love is best love.I love every single ultimate jutsu in Naruto Ultimate Ninja Storm (the first one). My favorite was Saskue's Chidori. It blew me away when I first saw it. All that lightning, and the way he just pulls his arm away is so cool. You can tell CC2 loved making this game.
The batclaw pull thing where Batman drags the bad guys towards him and punch them into the ground with his elbow in the Arkham games.